Publications
Readiness for the Cornell ERL
Energy-Recovery Linacs (ERLs) are proposed as drivers for hard x-ray sources because of their ability to produce electron bunches with small, flexible cross sections and short lengths at high repetition rates. Cornell University has pioneered the design and hardware for ERL lightsources. This preparatory research for ERL-lightsource construction will be discussed.
From damage percolation to crack nucleation through finite size criticality
We present a unified theory of fracture in disordered brittle media that reconciles apparently conflicting results reported in the literature. Our renormalization group based approach yields a phase diagram in which the percolation fixed point, expected for infinite disorder, is unstable for finite disorder and flows to a zero-disorder nucleation-type fixed point, thus showing that fracture has a mixed first order and continuous character. In a region of intermediate disorder and finite system sizes, we predict a crossover with mean-field avalanche scaling.
Magnetic-field dependence of Raman coupling in alkali-metal atoms
We calculate the magnetic-field dependence of Rabi rates for two-photon optical Raman processes in alkali-metal atoms. Due to a decoupling of the nuclear and electronic spins, these rates fall with increasing field. At the typical magnetic fields of alkali-metal-atom Feshbach resonances (B∼200-1200 G), the Raman rates have the same order of magnitude as their zero-field values, suggesting one can combine Raman-induced gauge fields or spin-orbital coupling with strong Feshbach-induced interactions.
Progress, challenges, and opportunities in two-dimensional materials beyond graphene
Graphene's success has shown that it is possible to create stable, single and few-atom-thick layers of van der Waals materials, and also that these materials can exhibit fascinating and technologically useful properties. Here we review the state-of-the-art of 2D materials beyond graphene. Initially, we will outline the different chemical classes of 2D materials and discuss the various strategies to prepare single-layer, few-layer, and multilayer assembly materials in solution, on substrates, and on the wafer scale.
Multicompartment mesoporous silica nanoparticles with branched shapes: An epitaxial growth mechanism
Mesoporous nanomaterials have attracted widespread interest because of their structural versatility for applications including catalysis, separation, and nanomedicine. We report a one-pot synthesis method for a class of mesoporous silica nanoparticles (MSNs) containing both cubic and hexagonally structured compartments within one particle. These multicompartment MSNs (mc-MSNs) consist of a core with cage-like cubic mesoporous morphology and up to four branches with hexagonally packed cylindrical mesopores epitaxially growing out of the cubic core vertices.
Regularization of the Coulomb singularity in exact exchange by Wigner-Seitz truncated interactions: Towards chemical accuracy in nontrivial systems
Hybrid density functionals show great promise for chemically accurate first-principles calculations, but their high computational cost limits their application in nontrivial studies, such as exploration of reaction pathways of adsorbents on periodic surfaces. One factor responsible for their increased cost is the dense Brillouin-zone sampling necessary to accurately resolve an integrable singularity in the exact exchange energy.
Magnetic polarons in two-component hard-core bosons
We use a high-temperature expansion to explore spin correlations around a single hole in a two-dimensional lattice filled with a hard-core two-component bose gas. We find that the spins around the hole develop ferromagnetic order and quantify the degree of polarization at temperatures of the order of the hopping energy, finding a measurably nonzero polarization. We also discuss the effect of fixing the overall magnetization of the system for finite-sized systems. © 2013 American Physical Society.
Anisotropic impurity states, quasiparticle scattering and nematic transport in underdoped Ca(Fe 1-x Co x ) 2 As 2
Iron-based high-temperature superconductivity develops when the 'parent' antiferromagnetic/orthorhombic phase is suppressed, typically by introduction of dopant atoms. But their impact on atomic-scale electronic structure, although in theory rather complex, is unknown experimentally. What is known is that a strong transport anisotropy with its resistivity maximum along the crystal b axis, develops with increasing concentration of dopant atoms; this 'nematicity'vanishes when the parent phase disappears near the maximum superconducting T c.
Orientation of luminescent excitons in layered nanomaterials
In nanomaterials, optical anisotropies reveal a fundamental relationship between structural and optical properties. Directional optical properties can be exploited to enhance the performance of optoelectronic devices, optomechanical actuators and metamaterials. In layered materials, optical anisotropies may result from in-plane and out-of-plane dipoles associated with intra- and interlayer excitations, respectively. Here, we resolve the orientation of luminescent excitons and isolate photoluminescence signatures arising from distinct intra- and interlayer optical transitions.
Teaching assistant professional development by and for TAs
In most large universities, much of the undergraduate teaching responsibility falls on graduate student teaching assistants (TAs), who are by then experienced students, but relatively inexperienced instructors. Institutions have a responsibility to offer quality instruction to undergraduate students and thus are responsible for preparing the TAs to teach.