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Publications

Thermodynamic constraints on the amplitude of quantum oscillations

Cornell Affiliated Author(s)
Author
Arkady Shekhter
K. Modic
R. McDonald
B. Ramshaw
Abstract

Magneto-quantum oscillation experiments in high-temperature superconductors show a strong thermally induced suppression of the oscillation amplitude approaching the critical dopings [B. J. Ramshaw, Science 348, 317 (2014)SCIEAS0036-807510.1126/science.aaa4990; H. Shishido, Phys. Rev. Lett. 104, 057008 (2010)PRLTAO0031-900710.1103/PhysRevLett.104.057008; P. Walmsley, Phys. Rev. Lett. 110, 257002 (2013)PRLTAO0031-900710.1103/PhysRevLett.110.257002] - in support of a quantum-critical origin of their phase diagrams.

Journal
Physical Review B
Date Published
Funding Source
PHY-1066293
DMR-1157490
1066293
1157490
Group (Lab)
Brad Ramshaw Group

Grand canonical electronic density-functional theory: Algorithms and applications to electrochemistry

Cornell Affiliated Author(s)
Author
R. Sundararaman
W.A. Goddard III
Tomas Arias
Abstract

First-principles calculations combining density-functional theory and continuum solvation models enable realistic theoretical modeling and design of electrochemical systems. When a reaction proceeds in such systems, the number of electrons in the portion of the system treated quantum mechanically changes continuously, with a balancing charge appearing in the continuum electrolyte. A grand-canonical ensemble of electrons at a chemical potential set by the electrode potential is therefore the ideal description of such systems that directly mimics the experimental condition.

Journal
Journal of Chemical Physics
Date Published
Funding Source
DE-SC0004993
DE-AC02-05CH11231
DE-SC0001086
Group (Lab)
Tomas Arias Group

Nanosecond magnetization dynamics during spin Hall switching of in-plane magnetic tunnel junctions

Cornell Affiliated Author(s)
Author
G. Rowlands
Sriharsha Aradhya
S. Shi
E. Yandel
J. Oh
D. Ralph
Robert Buhrman
Abstract

We present a study of the magnetic dynamics associated with nanosecond scale magnetic switching driven by the spin Hall effect in 3-terminal nanoscale magnetic tunnel junctions (MTJs) with in-plane magnetization.

Journal
AIP Publishing
Date Published
Funding Source
ECCS-0335765
0335765
W911NF-14-C0089
DMR-1120296

Surface atomic structure of epitaxial LaNiO3 thin films studied by in situ LEED- I(V)

Cornell Affiliated Author(s)
Author
J.P. Ruf
P.D.C. King
V.B. Nascimento
D.G. Schlom
K.M. Shen
Abstract

We report in situ low-energy electron diffraction intensity versus voltage [LEED-I(V)] studies of the surface atomic structure of epitaxially grown (001)pc-oriented (pc=pseudocubic) thin films of the correlated 3d transition-metal oxide LaNiO3. Our analysis indicates the presence of large out-of-plane bucklings of the topmost LaO layers but only minor bucklings of the topmost NiO2 layers, in close agreement with earlier surface x-ray diffraction data.

Journal
Physical Review B
Date Published
Funding Source
APQ-01961-14
DMR-1120296
DGE-0903653
N00014-12-1-0791
Group (Lab)
Kyle Shen Group

Influence of Surface Adsorption on the Oxygen Evolution Reaction on IrO2(110)

Cornell Affiliated Author(s)
Author
D.-Y. Kuo
J.K. Kawasaki
J.N. Nelson
J. Kloppenburg
G. Hautier
K.M. Shen
D.G. Schlom
J. Suntivich
Abstract

A catalyst functions by stabilizing reaction intermediates, usually through surface adsorption. In the oxygen evolution reaction (OER), surface oxygen adsorption plays an indispensable role in the electrocatalysis. The relationship between the adsorption energetics and OER kinetics, however, has not yet been experimentally measured. Herein we report an experimental relationship between the adsorption of surface oxygen and the kinetics of the OER on IrO2(110) epitaxially grown on a TiO2(110) single crystal.

Journal
Journal of the American Chemical Society
Date Published
Funding Source
DMR-1120296
DGE-1650441
ECCS-0335765
2.5020.11
Group (Lab)
Kyle Shen Group

Characterization and control of ZnGeN2 cation lattice ordering

Cornell Affiliated Author(s)
Author
E.W. Blanton
K. He
J. Shan
K. Kash
Abstract

ZnGeN2 and other heterovalent ternary semiconductors have important potential applications in optoelectronics, but ordering of the cation sublattice, which can affect the band gap, lattice parameters, and phonons, is not yet well understood. Here the effects of growth and processing conditions on the ordering of the ZnGeN2 cation sublattice were investigated using x-ray diffraction and Raman spectroscopy. Polycrystalline ZnGeN2 was grown by exposing solid Ge to Zn and NH3 vapors at temperatures between 758 °C and 914 °C.

Journal
Journal of Crystal Growth
Date Published
Funding Source
1006132
1106225
1409346
Group (Lab)
Jie Shan Group

Control of spin–orbit torques through crystal symmetry in WTe2/ferromagnet bilayers

Cornell Affiliated Author(s)
Author
D. Macneill
G. Stiehl
Marcos Guimarães
Robert Buhrman
J. Park
D. Ralph
Abstract

Recent discoveries regarding current-induced spin-orbit torques produced by heavy-metal/ferromagnet and topological-insulator/ferromagnet bilayers provide the potential for dramatically improved efficiency in the manipulation of magnetic devices. However, in experiments performed to date, spin-orbit torques have an important limitation - the component of torque that can compensate magnetic damping is required by symmetry to lie within the device plane.

Journal
Springer Science and Business Media LLC
Date Published
Funding Source
DGE-1144153
DMR-1120296
DMR-1539918
ECCS-1542081
NWO 680-50-1311
1406333
1539918
DMR-1406333
W911NF-15-1-0447
680-50-1311

Multiscale strain as a predictor of impact-induced fissuring in articular cartilage

Cornell Affiliated Author(s)
Author
C.R. Henak
L.R. Bartell
Itai Cohen
L.J. Bonassar
Abstract

Mechanical damage is central to both initiation and progression of osteoarthritis (OA). However, specific causal links between mechanics and cartilage damage are incompletely understood, which results in an inability to predict failure. The lack of understanding is primarily due to the difficulty in simultaneously resolving the high rates and small length scales relevant to the problem and in correlating such measurements to the resulting fissures.

Journal
Journal of Biomechanical Engineering
Date Published
Funding Source
1536463
-1144153
NSF DMR 1120296
R21AR062677
Group (Lab)
Itai Cohen Group

Theoretical estimates of maximum fields in superconducting resonant radio frequency cavities: Stability theory, disorder, and laminates

Cornell Affiliated Author(s)
Author
D.B. Liarte
S. Posen
M.K. Transtrum
G. Catelani
M. Liepe
J.P. Sethna
Abstract

Theoretical limits to the performance of superconductors in high magnetic fields parallel to their surfaces are of key relevance to current and future accelerating cavities, especially those made of new higher-T c materials such as Nb3Sn, NbN, and MgB2. Indeed, beyond the so-called superheating field , flux will spontaneously penetrate even a perfect superconducting surface and ruin the performance. We present intuitive arguments and simple estimates for , and combine them with our previous rigorous calculations, which we summarize.

Journal
Superconductor Science and Technology
Date Published
Funding Source
1312160
1416318
618258
Group (Lab)
James Sethna Group

Cooling quantum gases with entropy localization

Cornell Affiliated Author(s)
Author
F.N. Ünal
E.J. Mueller
Abstract

We study the dynamics of entropy in a time dependent potential and explore how disorder influences this entropy flow. We show that disorder can trap entropy at the edge of the atomic cloud enabling a novel cooling method. We demonstrate the feasibility of our cooling technique by analyzing the evolution of entropy in a one-dimensional Fermi lattice gas with a time dependent superlattice potential. © 2017 IOP Publishing Ltd and Deutsche Physikalische Gesellschaft.

Journal
New Journal of Physics
Date Published
Funding Source
1508300
PHY1508300