Publications
Ultrafast photocurrent measurement of the escape time of electrons and holes from carbon nanotube p-i-n photodiodes
Ultrafast photocurrent measurements are performed on individual carbon nanotube p-i-n photodiodes. The photocurrent response to subpicosecond pulses separated by a variable time delay Δt shows strong photocurrent suppression when two pulses overlap (Δt=0). The picosecond-scale decay time of photocurrent suppression scales inversely with the applied bias V SD, and is twice as long for photon energy above the second subband E 22 as compared to lower energy. The observed photocurrent behavior is well described by an escape time model that accounts for carrier effective mass.
Fracture strength of disordered media: Universality, interactions, and tail asymptotics
We study the asymptotic properties of fracture strength distributions of disordered elastic media by a combination of renormalization group, extreme value theory, and numerical simulation. We investigate the validity of the "weakest-link hypothesis" in the presence of realistic long-ranged interactions in the random fuse model. Numerical simulations indicate that the fracture strength is well-described by the Duxbury-Leath-Beale (DLB) distribution which is shown to flow asymptotically to the Gumbel distribution.
Terahertz imaging and time-domain spectroscopy of large-area graphene on silicon
We demonstrate THz imaging and time-domain spectroscopy of a single-layer graphene film. The large-area graphene was grown by chemical vapor deposition on Cu-foil and subsequently transferred to a Si substrate. We took a transmission image of the graphene/Si sample measured by a Si:bolometer (pixel size is 0.4-mm). The graphene film (transmission: 36 - 41%) is clearly resolved against the background of the Si substrate (average transmission: 56.6%). The strong THz absorption by the graphene layer indicates that THz carrier dynamics are dominated by intraband transitions.
Non-abelian braiding of lattice bosons
We report on a numerical experiment in which we use time-dependent potentials to braid non-Abelian quasiparticles. We consider lattice bosons in a uniform magnetic field within the fractional quantum Hall regime, where ν, the ratio of particles to flux quanta, is near 1/2, 1, or 3/2. We introduce time-dependent potentials which move quasiparticle excitations around one another, explicitly simulating a braiding operation which could implement part of a gate in a quantum computation.
Global radiation damage at 300 and 260 K with dose rates approaching 1 MGy s -1
Global radiation damage to 19 thaumatin crystals has been measured using dose rates from 3 to 680 kGy s -1. At room temperature damage per unit dose appears to be roughly independent of dose rate, suggesting that the timescales for important damage processes are less than ∼1 s. However, at T = 260 K approximately half of the global damage manifested at dose rates of 10 kGy s -1 can be outrun by collecting data at 680 kGy s -1. Appreciable sample-to-sample variability in global radiation sensitivity at fixed dose rate is observed.
Recent advances in single molecule studies of nucleosomes
As the fundamental packing units of DNA in eukaryotes, nucleosomes play a central role in governing DNA accessibility in a variety of cellular processes. Our understanding of the mechanisms underlying this complex regulation has been aided by unique structural and dynamic perspectives offered by single molecule techniques.
Dispersion and wave-function symmetry in cold atoms experiencing artificial gauge fields
We analyze the single-particle quantum mechanics of an atom whose dispersion is modified by spin-orbit coupling to Raman lasers. Such a setup can create a double-well-shaped dispersion, which leads to unusual single-particle physics. We show how this dispersion influences the symmetry of the ground-state wave function in different physical-space potentials, including a square well, a harmonic well, and a double well. © 2012 American Physical Society.
Time-resolved protein nanocrystallography using an X-ray free-electron laser
We demonstrate the use of an X-ray free electron laser synchronized with an optical pump laser to obtain X-ray diffraction snapshots from the photoactivated states of large membrane protein complexes in the form of nanocrystals flowing in a liquid jet. Light-induced changes of Photosystem I-Ferredoxin co-crystals were observed at time delays of 5 to 10 μs after excitation. The result correlates with the microsecond kinetics of electron transfer from Photosystem I to ferredoxin.
Networked and chiral nanocomposites from ABC triblock terpolymer coassembly with transition metal oxide nanoparticles
Multicomponent materials with ordered nanoscale networks are critical for applications ranging from microelectronics to energy conversion and storage devices which require charge transport along 3-dimensional (3D) continuous pathways. The network symmetry can facilitate additional properties such as macroscopic polarization for piezoelectric, pyroelectric, and second-order nonlinear optical properties in non-centrosymmetric morphologies. Although pure block copolymers are able to form multiple network morphologies, network tunability remains a challenge for coassembled systems.
Senescent cells in growing tumors: Population dynamics and cancer stem cells
Tumors are defined by their intense proliferation, but sometimes cancer cells turn senescent and stop replicating. In the stochastic cancer model in which all cells are tumorigenic, senescence is seen as the result of random mutations, suggesting that it could represent a barrier to tumor growth. In the hierarchical cancer model a subset of the cells, the cancer stem cells, divide indefinitely while other cells eventually turn senescent. Here we formulate cancer growth in mathematical terms and obtain predictions for the evolution of senescence.