Publications
Stirring trapped atoms into fractional quantum Hall puddles
We theoretically explore the generation of few-body analogs of fractional quantum Hall states. We consider an array of identical few-atom clusters (n=2,3,4), each cluster trapped at the node of an optical lattice. By temporally varying the amplitude and phase of the trapping lasers, one can introduce a rotating deformation at each site. We analyze protocols for coherently transferring ground-state clusters into highly correlated states, producing theoretical fidelities (probability of reaching the target state) in excess of 99%. © 2008 The American Physical Society.
High temperature electrical resistance of substrate-supported single walled carbon nanotubes
We report the electrical characteristics of substrate-supported metallic single walled carbon nanotubes at temperatures up to 573 K over a range of bias voltages (Vb) for zero gate voltage in air under atmospheric pressure. Our results show a monotonic increase in resistance with temperature, with an I- Vb characteristic that is linear at high temperature but nonlinear at low temperature.
Temperature dependence of the superheating field for superconductors in the high-κ London limit
We study the metastability of the superheated Meissner state in type II superconductors with κ≫1 beyond Ginzburg-Landau theory, which is applicable only in the vicinity of the critical temperature. Within Eilenberger's semiclassical approximation, we use the local electrodynamic response of the superconductor to derive a generalized thermodynamic potential valid at any temperature. The stability analysis of this functional yields the temperature dependence of the superheating field.
Bogoliubov angle and visualization of particle-hole mixture in superconductors
Superconducting excitations-Bogoliubov quasiparticles-are the quantum mechanical mixture of negatively charged electron (-e) and positively charged hole (+e). Depending on the applied voltage bias in scanning tunneling microscope (STM) one can sample the particle and hole content of such a superconducting excitation. Recent STM experiments offer a unique insight into the inner workings of the superconducting state of superconductors. We propose a new observable quantity for STM studies that is the manifestation of the particle-hole dualism of the quasiparticles.
Graphene as an electronic membrane
We investigate the membrane aspect of graphene and its impact on the electronic properties. We show that rippling generates spatially varying electrochemical potential that is proportional to the square of the local curvature. This is due to the rehybridization effects and the change in the next-neighbor hopping caused by curvature. We estimate the electrochemical- potential variation associated with the rippling observed in recent scanning tunneling microscopy (STM) to be of order 30 meV. Further we show that the charge inhomogeneity in turn stabilizes ripple formation.
Quantum Monte Carlo study of the cooperative binding of NO2 to fragment models of carbon nanotubes
Previous calculations on model systems for the cooperative binding of two NO2 molecules to carbon nanotubes using density functional theory and second order Moller-Plesset perturbation theory gave results differing by 30 kcal/mol. Quantum Monte Carlo calculations are performed to study the role of electronic correlations in these systems and resolve the discrepancy between these previous calculations. Compared to QMC binding energies, MP2 and LDA are shown to overbind, while B3LYP and BPW91 underbind.
Kohn-Sham-like approach toward a classical density-functional theory of inhomogeneous polar molecular liquids: An application to liquid hydrogen chloride
The Gordian knot of density-functional theories for classical molecular liquids remains finding an accurate free-energy functional in terms of the densities of the atomic sites of the molecules. Following Kohn and Sham, we show how to solve this problem by considering noninteracting molecules in a set of effective potentials. This shift in perspective leads to an accurate and computationally tractable description in terms of simple three-dimensional functions.
High resolution shear profile measurements in entangled polymers
We use confocal microscopy and particle image velocimetry to visualize motion of 250-300 nm. fluorescent tracer particles in entangled polymers subject to a rectilinear shear flow. Our results show linear velocity profiles in polymer solutions spanning a wide range of molecular weights and number of entanglements (8≤Z≤56), but reveal large differences between the imposed and measured shear rates. These findings disagree with recent reports that shear banding is a characteristic flow response of entangled polymers, and instead point to interfacial slip as an important source of strain loss.
Stability of bosonic atomic and molecular condensates near a Feshbach resonance
We explore the Bose condensed phases of an atomic gas on the molecular side of a Feshbach resonance. In the absence of atom-molecule and molecule-molecule scattering, we show that the atomic condensate is either a saddle point of the free energy with energy always exceeding that of the molecular condensate, or has a negative compressibility (hence unstable to density fluctuations). Therefore no phase transition occurs between the atomic and molecular condensates.
Liquid interfaces in viscous straining flows: Numerical studies of the selective withdrawal transition
This paper presents a numerical analysis of the transition from selective withdrawal to viscous entrainment. In our model problem, an interface between two immiscible layers of equal viscosity is deformed by an axisymmetric withdrawal flow, which is driven by a point sink located some distance above the interface in the upper layer. We find that steady-state hump solutions, corresponding to selective withdrawal of liquid from the upper layer, cease to exist above a threshold withdrawal flux, and that this transition corresponds to a saddle-node bifurcation for the hump solutions.