Publications
Controlling carbon nanotube mechanics with optical microcavities
We demonstrate optomechanically induced amplification of carbon nanotube (CNT) mechanical modes using optical microcavities. We also show direct imaging of the spatial profile of CNT mechanical modes using optical readout. © 2015 OSA.
Graphene kirigami
For centuries, practitioners of origami ( ori, fold; kami, paper) and kirigami ( kiru, cut) have fashioned sheets of paper into beautiful and complex three-dimensional structures. Both techniques are scalable, and scientists and engineers are adapting them to different two-dimensional starting materials to create structures from the macro- to the microscale1,2. Here we show that graphene3-6 is well suited for kirigami, allowing us to build robust microscale structures with tunable mechanical properties.
Folded graphene nanochannels via pulsed patterning of graphene
We present a resist-free patterning technique to form electrically contacted graphene nanochannels via localized burning by a pulsed white light source. The technique uses end-point detection to stop the burning process at a fixed resistance to produce channels with resistances of 10 kΩ to 100 kΩ. Folding of the graphene sheet takes place during patterning, which provides very straight edges as identified by AFM and SEM.
Coupling of plasmon modes in graphene microstructures
A variety of different graphene plasmonic structures and devices have been proposed and demonstrated experimentally. Plasmon modes in graphene microstructures interact strongly via the depolarization fields. An accurate quantitative description of the coupling between plasmon modes is required for designing and understanding complex plasmonic devices. Drawing inspiration from microphotonics, we present a coupled-mode theory for graphene plasmonics, in which the plasmon eigenmodes of a coupled system are expressed in terms of the plasmon eigenmodes of its uncoupled sub-systems.
Atomic imaging across strain boundaries in bilayer graphene with ADF-STEM and DF-TEM
The valley hall effect in MoS2 transistors
Electrons in two-dimensional crystals with a honeycomb lattice structure possess a valley degree of freedom (DOF) in addition to charge and spin. These systems are predicted to exhibit an anomalous Hall effect whose sign depends on the valley index. Here, we report the observation of this so-called valley Hall effect (VHE). Monolayer MoS2 transistors are illuminated with circularly polarized light, which preferentially excites electrons into a specific valley, causing a finite anomalous Hall voltage whose sign is controlled by the helicity of the light.
Cavity optomechanics with suspended carbon nanotubes
We demonstrate large optomechanical coupling between a carbon nanotube and an optical microresonator. We measured a dominantly dissipative optomechanical coupling coefficient of gk = 1 MHz/nm. © 2014 Optical Society of America.
Stacking order dependent second harmonic generation and topological defects in h-BN bilayers
The ability to control the stacking structure in layered materials could provide an exciting approach to tuning their optical and electronic properties. Because of the lower symmetry of each constituent monolayer, hexagonal boron nitride (h-BN) allows more structural variations in multiple layers than graphene; however, the structure-property relationships in this system remain largely unexplored.
Transient absorption and photocurrent microscopy show that hot electron supercollisions describe the rate-limiting relaxation step in graphene
Using transient absorption (TA) microscopy as a hot electron thermometer, we show that disorder-assisted acoustic-phonon supercollisions (SCs) best describe the rate-limiting relaxation step in graphene over a wide range of lattice temperatures (Tl = 5-300 K), Fermi energies (EF = ± 0.35 eV), and optical probe energies (∼0.3-1.1 eV). Comparison with simultaneously collected transient photocurrent, an independent hot electron thermometer, confirms that the rate-limiting optical and electrical response in graphene are best described by the SC-heat dissipation rate model, H = A(T e3 - Tl3).
Imaging atomic rearrangements in two-dimensional silica glass: Watching silica's dance
Structural rearrangements control a wide range of behavior in amorphous materials, and visualizing these atomic-scale rearrangements is critical for developing and refining models for how glasses bend, break, and melt. It is difficult, however, to directly image atomic motion in disordered solids. We demonstrate that using aberration-corrected transmission electron microscopy, we can excite and image atomic rearrangements in a two-dimensional silica glass - revealing a complex dance of elastic and plastic deformations, phase transitions, and their interplay.