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Publications

Comparing Thickness and Doping-Induced Effects on the Normal States of Infinite-Layer Electron-Doped Cuprates: Is There Anything to Learn?

Cornell Affiliated Author(s)
Author
C. Sacco
A. Galdi
F. Romeo
N. Coppola
P. Orgiani
H.I. Wei
K.M. Shen
D.G. Schlom
L. Maritato
Abstract

We grew Sr1−xLaxCuO2 thin films and SrCuO2/Sr0.9La0.1CuO2/SrCuO2 trilayers by reflection high-energy diffraction-calibrated layer-by-layer molecular beam epitaxy, to study their electrical transport properties as a function of the doping and thickness of the central Sr0.9La0.1CuO2 layer.

Journal
Nanomaterials
Date Published
Group (Lab)
Kyle Shen Group

Strong interlayer interactions in bilayer and trilayer moire superlattices

Author
S. Xie
B.D. Faeth
Y. Tang
L. Li
E. Gerber
C.T. Parzyck
Debanjan Chowdhury
Y.-H. Zhang
C. Jozwiak
A. Bostwick
E. Rotenberg
Eun-Ah Kim
J. Shan
K.F. Mak
K.M. Shen
Abstract

Moire superlattices constructed from transition metal dichalcogenides have demonstrated a series of emergent phenomena, including moire excitons, flat bands, and correlated insulating states. All of these phenomena depend crucially on the presence of strong moire potentials, yet the properties of these moire potentials, and the mechanisms by which they can be generated, remain largely open questions. Here, we use angle-resolved photoemission spectroscopy with submicron spatial resolution to investigate an aligned WS2/WSe2moire superlattice and graphene/WS2/WSe2trilayer heterostructure.

Journal
Science Advances
Date Published
Group (Lab)
Debanjan Chowdhury Group
Jie Shan Group
Kin Fai Mak Group
Kyle Shen Group

Single-Crystal Alkali Antimonide Photocathodes: High Efficiency in the Ultrathin Limit

Cornell Affiliated Author(s)
Author
C.T. Parzyck
A. Galdi
J.K. Nangoi
W.J.I. Debenedetti
J. Balajka
B.D. Faeth
H. Paik
C. Hu
Tomas Arias
M.A. Hines
D.G. Schlom
K.M. Shen
J.M. Maxson
Abstract

The properties of photoemission electron sources determine the ultimate performance of a wide class of electron accelerators and photon detectors. To date, all high-efficiency visible-light photocathode materials are either polycrystalline or exhibit intrinsic surface disorder, both of which limit emitted electron beam brightness. In this Letter, we demonstrate the synthesis of epitaxial thin films of Cs3Sb on 3C-SiC (001) using molecular-beam epitaxy. Films as thin as 4 nm have quantum efficiencies exceeding 2% at 532 nm.

Journal
Physical Review Letters
Date Published
Funding Source
DMR-2039380
PHY-1549132
DMR-1719875
DMR-2104427
Group (Lab)
Kyle Shen Group
Tomas Arias Group

Interfacial charge transfer and persistent metallicity of ultrathin SrIrO3/SrRuO3 heterostructures

Cornell Affiliated Author(s)
Author
J.N. Nelson
N.J. Schreiber
A.B. Georgescu
B.H. Goodge
B.D. Faeth
C.T. Parzyck
Cyrus Zeledon
L.F. Kourkoutis
A.J. Millis
A. Georges
D.G. Schlom
K.M. Shen
Abstract

Interface quantum materials have yielded a plethora of previously unknown phenomena, including unconventional superconductivity, topological phases, and possible Majorana fermions. Typically, such states are detected at the interface between two insulating constituents by electrical transport, but whether either material is conducting, transport techniques become insensitive to interfacial properties.

Journal
Science Advances
Date Published
Group (Lab)
Kyle Shen Group

Computational synthesis of substrates by crystal cleavage

Cornell Affiliated Author(s)
Author
J.T. Paul
A. Galdi
C. Parzyck
K. Shen
J. Maxson
R.G. Hennig
Abstract

The discovery of substrate materials has been dominated by trial and error, opening the opportunity for a systematic search. We generate bonding networks for materials from the Materials Project and systematically break up to three bonds in the networks for three-dimensional crystals. Successful cleavage reduces the bonding network to two periodic dimensions. We identify 4693 symmetrically unique cleavage surfaces across 2133 bulk crystals, 4626 of which have a maximum Miller index of one.

Journal
npj Computational Materials
Date Published
Funding Source
DMR-1542776
DMS-1440415
OAC-1740251
PHY-1549132
Group (Lab)
Kyle Shen Group

THz electrodynamics of mixed-valent YbAl 3 and LuAl 3 thin films

Cornell Affiliated Author(s)
Author
D. Barbalas
S. Chatterjee
D.G. Schlom
K.M. Shen
N.P. Armitage
Abstract

We present our results from time-domain THz spectroscopy measurements of thin films of mixed-valent YbAl3 and its structural analogue LuAl3. Combined with Fourier transform infrared (FTIR) spectroscopy, the extended Drude formalism is utilized to study the quasiparticle scattering rate and effective masses in YbAl3. We find that LuAl3 demonstrates conventional Drude transport whereas at low temperatures YbAl3 demonstrates a renormalized Drude peak and a mid-infrared (MIR) peak in the conductivity, indicative of the formation of a mass-enhanced Fermi liquid (FL).

Journal
European Physical Journal B
Date Published
Funding Source
DMR-1539918
DMR-170925
ECCS-1542081
FA9550-15-1-0474
90088577
Group (Lab)
Kyle Shen Group

Vanishing nematic order beyond the pseudogap phase in overdoped cuprate superconductors

Cornell Affiliated Author(s)
Author
N.K. Gupta
C. McMahon
R. Sutarto
T. Shi
R. Gong
H.I. Wei
K.M. Shen
F. He
Q. Ma
M. Dragomir
B.D. Gaulin
D.G. Hawthorn
Abstract

During the last decade, translational and rotational symmetry-breaking phases—density wave order and electronic nematicity—have been established as generic and distinct features of many correlated electron systems, including pnictide and cuprate superconductors. However, in cuprates, the relationship between these electronic symmetry-breaking phases and the enigmatic pseudogap phase remains unclear.

Journal
Proceedings of the National Academy of Sciences of the United States of America
Date Published
Funding Source
FA9550-15-1-0474
FA9550-21-1-0168
Group (Lab)
Kyle Shen Group

Quantum oscillations and quasiparticle properties of thin film

Cornell Affiliated Author(s)
Author
Yawen Fang
Hari Nair
Ludi Miao
Berit Goodge
Nathaniel Schreiber
Jacob Ruf
Lena Kourkoutis
Kyle Shen
Darrell Schlom
B. Ramshaw
Abstract

We measure the Shubnikov-de Haas effect in thin-film grown on an substrate. We detect all three known Fermi surfaces and extract the Fermi surface volumes, cyclotron effective masses, and quantum lifetimes. We show that the electronic structure is nearly identical to that of single-crystal , and that the quasiparticle lifetime is consistent with the of comparably clean, single-crystal . Unlike single-crystal , where the quantum and transport lifetimes are roughly equal, we find that the transport lifetime is times longer than the quantum lifetime.

Journal
Physical Review B
Date Published
Funding Source
DMR-1709255
DGE-1650441
DMR-1539918
1429155
DMR-1644779
DMR-1752784
NNCI-2025233
FA9550-15-1-0474
GBMF3850
GBMF9073
DMR-1719875
Group (Lab)
Brad Ramshaw Group
Kyle Shen Group

Interfacial Electron-Phonon Coupling Constants Extracted from Intrinsic Replica Bands in Monolayer FeSe/SrTi O3

Cornell Affiliated Author(s)
Author
B.D. Faeth
S. Xie
S. Yang
J.K. Kawasaki
J.N. Nelson
S. Zhang
C. Parzyck
P. Mishra
C. Li
C. Jozwiak
A. Bostwick
E. Rotenberg
D.G. Schlom
K.M. Shen
Abstract

The observation of replica bands by angle-resolved photoemission spectroscopy has ignited interest in the study of electron-phonon coupling at low carrier densities, particularly in monolayer FeSe/SrTiO3, where the appearance of replica bands has motivated theoretical work suggesting that the interfacial coupling of electrons in the FeSe layer to optical phonons in the SrTiO3 substrate might contribute to the enhanced superconducting pairing temperature.

Journal
Physical Review Letters
Date Published
Funding Source
DMR-1539918
DMR-1709255
FA9550-15-1-0474
FA9550-21-1-0168
DGE-1650441
GBMF3850
DE-AC02-05CH11231
ECCS-1542081
DMR-1719875
Group (Lab)
Kyle Shen Group

Incoherent Cooper Pairing and Pseudogap Behavior in Single-Layer FeSe/SrTi O3

Cornell Affiliated Author(s)
Author
B.D. Faeth
S.-L. Yang
J.K. Kawasaki
J.N. Nelson
P. Mishra
C.T. Parzyck
C. Li
D.G. Schlom
K.M. Shen
Abstract

In many unconventional superconductors, the presence of a pseudogap - a suppression in the electronic density of states extending above the critical temperature - has been a long-standing mystery. Here, we employ combined in situ electrical transport and angle-resolved photoemission spectroscopy measurements to reveal an unprecedentedly large pseudogap regime in single-layer FeSe/SrTiO3, an interfacial superconductor where incoherent Cooper pairs are initially formed above TΔ≈60 K but where a zero-resistance state is achieved only below T0<30 K.

Journal
Physical Review X
Date Published
Funding Source
1709255
DMR-1539918
DMR-1709255
FA9550-15-1-0474
FA9550-21-1-0168
DGE-1650441
GBMF3850
DMR-1719875
ECCS-1542081
Group (Lab)
Kyle Shen Group