Publications
Quasiparticle mass enhancement and temperature dependence of the electronic structure of ferromagnetic SrRuO3 thin films
We report high-resolution angle-resolved photoemission studies of epitaxial thin films of the correlated 4d transition metal oxide ferromagnet SrRuO 3. The Fermi surface in the ferromagnetic state consists of well-defined Landau quasiparticles exhibiting strong coupling to low-energy bosonic modes which contributes to the large effective masses observed by transport and thermodynamic measurements.
Layer-by-layer shuttered molecular-beam epitaxial growth of superconducting Sr1-xLaxCuO2 thin films
Superconducting Sr1-xLaxCuO2 thin films have been grown on GdScO3 substrates by reflection high-energy electron diffraction calibrated layer-by-layer molecular-beam epitaxy. X-ray diffraction analysis has confirmed the infinite layer structure after an in situ vacuum annealing step. In situ photoemission spectroscopy indicates that the vacuum annealing step employed immediately after film growth to achieve superconducting films results in oxygen loss from the films. The superconducting critical temperature depends on the La content x, with the highest value obtained for x ∼ 0.10.
Nodeless superconducting phase arising from a strong (π, π) antiferromagnetic phase in the infinite-layer electron-doped sr 1-xlaxcuo2 compound
The asymmetry between electron and hole doping remains one of the central issues in high-temperature cuprate superconductivity, but our understanding of the electron-doped cuprates has been hampered by apparent discrepancies between the only two known families: Re2-xCexCuO4 and A1-xLaxCuO2. Here we report in situ angle-resolved photoemission spectroscopy measurements of epitaxially stabilized Sr1-xLaxCuO2 thin films synthesized by oxide molecular-beam epitaxy.
A tunable low-energy photon source for high-resolution angle-resolved photoemission spectroscopy
We describe a tunable low-energy photon source consisting of a laser-driven xenon plasma lamp coupled to a Czerny-Turner monochromator. The combined tunability, brightness, and narrow spectral bandwidth make this light source useful in laboratory-based high-resolution photoemission spectroscopy experiments. The source supplies photons with energies up to ∼7 eV, delivering under typical conditions >1012 ph/s within a 10 meV spectral bandwidth, which is comparable to helium plasma lamps and many synchrotron beamlines.
Quantum many-body interactions in digital oxide superlattices
Controlling the electronic properties of interfaces has enormous scientific and technological implications and has been recently extended from semiconductors to complex oxides that host emergent ground states not present in the parent materials. These oxide interfaces present a fundamentally new opportunity where, instead of conventional bandgap engineering, the electronic and magnetic properties can be optimized by engineering quantum many-body interactions.
Temperature dependence of the electronic structure and Fermi-surface reconstruction of Eu 1-xGd xO through the ferromagnetic metal-insulator transition
We present angle-resolved photoemission spectroscopy of Eu 1-xGd xO through the ferromagnetic metal-insulator transition. In the ferromagnetic phase, we observe Fermi surface pockets at the Brillouin zone boundary, consistent with density functional theory, which predicts a half-metal. Upon warming into the paramagnetic state, our results reveal a strong momentum-dependent evolution of the electronic structure, where the metallic states at the zone boundary are replaced by pseudogapped states at the Brillouin zone center due to the absence of magnetic long-range order of the Eu 4f moments.
Lutetium-doped EuO films grown by molecular-beam epitaxy
The effect of lutetium doping on the structural, electronic, and magnetic properties of epitaxial EuO thin films grown by reactive molecular-beam epitaxy is experimentally investigated. The behavior of Lu-doped EuO is contrasted with doping by lanthanum and gadolinium. All three dopants are found to behave similarly despite differences in electronic configuration and ionic size. Andreev reflection measurements on Lu-doped EuO reveal a spin-polarization of 96% in the conduction band, despite non-magnetic carriers introduced by 5% lutetium doping. © 2012 American Institute of Physics.
Determination of total X-ray absorption coefficient using non-resonant X-ray emission
An alternative measure of X-ray absorption spectroscopy (XAS) called inverse partial fluorescence yield (IPFY) has recently been developed that is both bulk sensitive and free of saturation effects. Here we show that the angle dependence of IPFY can provide a measure directly proportional to the total X-ray absorption coefficient, μ(E). In contrast, fluorescence yield (FY) and electron yield (EY) spectra are offset and/or distorted from μ(E) by an unknown and difficult to measure amount.
Polaronic metal in lightly doped high-Tc cuprates
We present a combined study of the angle-resolved-photoemission spectroscopy (ARPES) and quantum Monte Carlo simulations to propose a novel polaronic metallic state in underdoped cuprates. An approximation scheme is proposed to represent underdoped cuprates away from 1/2 filling, replacing the many-body Hamiltonian by that of a single polaron with effective electron-phonon interaction (EPI), that successfully explains many puzzles such as a large momentum-dependent dichotomy between nodal and antinodal directions, and an unconventional doping dependence of ARPES in the underdoped region.
Resonant elastic soft x-ray scattering in oxygen-ordered YBa 2Cu3O6+δ
Static charge-density-wave (CDW) and spin-density-wave (SDW) order has been convincingly observed in La-based cuprates for some time. However, more recently it has been suggested by quantum oscillation, transport, and thermodynamic measurements that density-wave order is generic to underdoped cuprates and plays a significant role in YBa2Cu3O 6+δ (YBCO). We use resonant soft x-ray scattering at the Cu L and O K edges to search for evidence of density-wave order in ortho-II and ortho-VIII oxygen-ordered YBCO.