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Observation of spin polarons in a frustrated moiré Hubbard system

Cornell Affiliated Author(s)

Author

Zui Tao
Wenjin Zhao
Bowen Shen
Tingxin Li
Patrick Knüppel
Kenji Watanabe
Takashi Taniguchi
Jie Shan
Kin Mak

Abstract

The electron’s kinetic energy plays a pivotal role in magnetism. While virtual electron hopping promotes antiferromagnetism in an insulator, real hopping processes usually favour ferromagnetism. However, in kinetically frustrated systems such as hole-doped triangular lattice Mott insulators, real hopping has instead been shown to favour antiferromagnetism. Kinetic frustration has also been predicted to induce a new quasiparticle, a bound state of the doped hole and a spin flip called a spin polaron, at intermediate magnetic fields, which could form an unusual metallic state. Here we report the direct observation of spin polarons in triangular lattice MoTe2/WSe2 moiré bilayers. A spin polaron phase emerges at a lattice filling factor just below 1 and is separated from the fully spin-polarized phase by a metamagnetic transition. We determine that the spin polaron is a spin-3/2 particle and that its binding energy is commensurate with the kinetic hopping energy. Our results will enable the exploration of spin polaron pseudogap metals, spin polaron pairing and other new phenomena in triangular lattice moiré materials.

Date Published

Journal

Nature Physics

ISBN Number

1745-2481

URL

https://doi.org/10.1038/s41567-024-02434-y

DOI

10.1038/s41567-024-02434-y

Group (Lab)

Jie Shan Group
Kin Fai Mak Group

Funding Source

FA9550-19-1-0390
DE-SC0019481
DMR-1807810
JPMJCR15F3
NNCI-2025233

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