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An algorithm for subtraction of doublet emission lines in angle-resolved photoemission spectroscopy

Cornell Affiliated Author(s)

Author

Y. Tarn
M. Sinha
C. Pasco
D.G. Schlom
T.M. McQueen
K.M. Shen
B.D. Faeth

Abstract

Plasma discharge lamps are widely utilized in the practice of angle-resolved photoemission spectroscopy (ARPES) experiments as narrow-linewidth ultraviolet photon sources. However, many emission lines such as Ar-I, Ne-I, and Ne-II have closely spaced doublet emission lines, which result in superimposed replica on the measured ARPES spectra. Here, we present a simple method for subtracting the contribution of these doublet emission lines from photoemission spectra. Benchmarking against ARPES spectra of well-characterized 2D materials, we demonstrate that this algorithm manages to subtract the doublet signal and reproduce the key features of the monochromated He-Iα spectra in a physically sound manner that reliably reproduces quantifiable dispersion relations and quasiparticle lifetimes. © 2023 Elsevier B.V.

Date Published

Journal

Journal of Electron Spectroscopy and Related Phenomena

Volume

265

URL

https://www.scopus.com/inward/record.uri?eid=2-s2.0-85159315090&doi=10.1016%2fj.elspec.2023.147323&partnerID=40&md5=68f18ec9d81885b54e3aa08bb844acee

DOI

10.1016/j.elspec.2023.147323

Group (Lab)

Kyle Shen Group

Funding Source

2039380

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