Skip to main content

Spectroscopic indications of polaronic behavior of the strong spin-orbit insulator Sr3Ir2O7

Cornell Affiliated Author(s)

Author

P.D.C. King
T. Takayama
A. Tamai
E. Rozbicki
S.M. Walker
M. Shi
L. Patthey
R.G. Moore
D. Lu
K.M. Shen
H. Takagi
F. Baumberger

Abstract

We investigate the bilayer Ruddlesden-Popper iridate Sr3Ir 2O7 by temperature-dependent angle-resolved photoemission. At low temperatures, we find a fully gapped correlated insulator, characterized by a small charge gap and narrow bandwidths. The low-energy spectral features show a pronounced temperature-dependent broadening and non-quasiparticle-like Gaussian line shapes. Together, these spectral features provide experimental evidence for a polaronic ground state. We observe similar behavior for the single-layer cousin Sr2IrO4, indicating that strong electron-boson coupling dominates the low-energy excitations of this exotic family of 5d compounds. © 2013 American Physical Society.

Date Published

Journal

Physical Review B - Condensed Matter and Materials Physics

Volume

87

Issue

24

URL

https://www.scopus.com/inward/record.uri?eid=2-s2.0-84879934007&doi=10.1103%2fPhysRevB.87.241106&partnerID=40&md5=4a5e1ed754b39909b260c7433190394d

DOI

10.1103/PhysRevB.87.241106

Group (Lab)

Kyle Shen Group

Funding Source

EP/I031014/1
24224010

Download citation