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Strongly correlated excitonic insulator in atomic double layers

Cornell Affiliated Author(s)

Author

L. Ma
P.X. Nguyen
Z. Wang
Y. Zeng
K. Watanabe
T. Taniguchi
A.H. MacDonald
K.F. Mak
J. Shan

Abstract

Excitonic insulators (EIs) arise from the formation of bound electron–hole pairs (excitons)1,2 in semiconductors and provide a solid-state platform for quantum many-boson physics3–8. Strong exciton–exciton repulsion is expected to stabilize condensed superfluid and crystalline phases by suppressing both density and phase fluctuations8–11. Although spectroscopic signatures of EIs have been reported6,12–14, conclusive evidence for strongly correlated EI states has remained elusive. Here we demonstrate a strongly correlated two-dimensional (2D) EI ground state formed in transition metal dichalcogenide (TMD) semiconductor double layers. A quasi-equilibrium spatially indirect exciton fluid is created when the bias voltage applied between the two electrically isolated TMD layers is tuned to a range that populates bound electron–hole pairs, but not free electrons or holes15–17. Capacitance measurements show that the fluid is exciton-compressible but charge-incompressible—direct thermodynamic evidence of the EI. The fluid is also strongly correlated with a dimensionless exciton coupling constant exceeding 10. We construct an exciton phase diagram that reveals both the Mott transition and interaction-stabilized quasi-condensation. Our experiment paves the path for realizing exotic quantum phases of excitons8, as well as multi-terminal exciton circuitry for applications18–20. © 2021, The Author(s), under exclusive licence to Springer Nature Limited.

Date Published

Journal

Nature

Volume

598

Issue

7882

Number of Pages

585-589,

URL

https://www.scopus.com/inward/record.uri?eid=2-s2.0-85117892345&doi=10.1038%2fs41586-021-03947-9&partnerID=40&md5=7dd36e4f48b60b4bfd2b3f522dd98a7b

DOI

10.1038/s41586-021-03947-9

Group (Lab)

Jie Shan Group
Kin Fai Mak Group

Funding Source

DMR-2004451
N00014-21-1-2471
DE-SC0019481
DE-SC0022058
NNCI-2025233
JPMJCR15F3

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