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The role of electron-phonon interactions on the coherence lifetime of monolayer transition metal dichalcogenides

Cornell Affiliated Author(s)

Author

C.E. Stevens
P. Dey
J. Paul
Z. Wang
H. Zhang
A.H. Romero
J. Shan
D.J. Hilton
D. Karaiskaj

Abstract

We investigate the excitonic dephasing of transition metal dichalcogenides, namely MoS2, MoSe2 and WSe2 atomic monolayer thick and bulk crystals, in order to understand the factors that determine the optical coherence in these materials. Coherent nonlinear optical spectroscopy, temperature dependent absorption combined with theoretical calculations of the phonon spectra, reveal the important role electron-phonon interactions plat in dephasing process. The temperature dependence of the electronic band gap and the excitonic linewidth combined with 'ab initio' calculations of the phonon energies and the phonon density of state reveal strong interaction with the E' and E" phonon modes.

Date Published

Conference Name

Journal of Physics: Conference Series

Publisher

IOP Publishing

URL

https://www.scopus.com/inward/record.uri?eid=2-s2.0-85028764793&doi=10.1088%2f1742-6596%2f864%2f1%2f012035&partnerID=40&md5=9cb8949f3f30f833219bb90ef009d1f3

DOI

10.1088/1742-6596/864/1/012035

Group (Lab)

Jie Shan Group

Funding Source

1434897
ACI-1053575
54075-ND10
DE-SC0012635

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