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Evolution of interlayer and intralayer magnetism in three atomically thin chromium trihalides

Cornell Affiliated Author(s)

Author

H.H. Kim
B. Yang
S. Li
S. Jiang
C. Jin
Z. Tao
G. Nichols
F. Sfigakis
S. Zhong
C. Li
S. Tian
D.G. Cory
G.-X. Miao
J. Shan
K.F. Mak
H. Lei
K. Sun
L. Zhao
A.W. Tsen

Abstract

We conduct a comprehensive study of three different magnetic semiconductors, CrI3, CrBr3, and CrCl3, by incorporating both few-layer and bilayer samples in van der Waals tunnel junctions. We find that the interlayer magnetic ordering, exchange gap, magnetic anisotropy, and magnon excitations evolve systematically with changing halogen atom. By fitting to a spin wave theory that accounts for nearest-neighbor exchange interactions, we are able to further determine a simple spin Hamiltonian describing all three systems. These results extend the 2D magnetism platform to Ising, Heisenberg, and XY spin classes in a single material family. Using magneto-optical measurements, we additionally demonstrate that ferromagnetism can be stabilized down to monolayer in more isotropic CrBr3, with transition temperature still close to that of the bulk. © 2019 National Academy of Sciences. All rights reserved.

Date Published

Journal

Proceedings of the National Academy of Sciences of the United States of America

Volume

166

Issue

23

Number of Pages

11131-11136,

URL

https://www.scopus.com/inward/record.uri?eid=2-s2.0-85066637370&doi=10.1073%2fpnas.1902100116&partnerID=40&md5=2d764a8600312f8229a0c40c7c62f357

DOI

10.1073/pnas.1902100116

Group (Lab)

Jie Shan Group
Kin Fai Mak Group

Funding Source

1749774
1807810
DMR-1749774
DMR-1807810
N00014-18-1-2368
ER17-13-199
RGPIN-2017-03815
11574394
11774423
11822412
NRF-2017K1A3A1A12073407
RGPIN-04178
2016YFA0300504

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