Atomically Resolved and Single Molecule Imaging, Spectroscopy, Dynamics, and Chemistry.

 

This material is based upon work supported by the following agencies.

Cornell Center for Materials Research through the National Science Foundation under Grant No. DMR-9632275.
National Science Foundation under Grant No. DMR-9417866, DMR-9707195.
U.S. Department of Energy, Division of Chemical Sciences, Office of Basic Energy Sciences, Office of Energy Research under Grant No. DMR-FG-02-91ER14205.

A Variable-Temperature Scanning Tunneling Microscope Capable of Single-Molecule Vibrational Spectroscopy, B.C. Stipe, M.A. Rezaei, and W. Ho, Rev. Sci. Instrum.70, 137-143 (1999).



Single Molecule Dissociation by Tunneling Electrons, B.C. Stipe, M.A. Rezaei, W. Ho, S. Gao, M. Persson, and B.I. Lundqvist, Phys. Rev. Lett. 78, 4410-4413 (1997).



O2 on Pt (111)

Inducing and Viewing the Rotational Motion of a Single Molecule, B.C. Stipe, M.A. Rezaei, and W. Ho, Science 279, 1907-1909 (1998).



Single Molecule Vibrational Spectroscopy and Microscopy, B.C. Stipe, M.A. Rezaei, and W. Ho, Science 280, 1732-1735 (1998).



Coupling of Vibrational Excitation to the Rotational Motion of a Single Adsorbed Molecule, B.C. Stipe, M.A. Rezaei, and W. Ho, Phys. Rev. Lett. 81, 1263-1266 (1998).



Localization of Inelastic Tunneling and the Determination of Atomic-Scale Structure with Chemical Sensitivity, B.C. Stipe, M.A. Rezaei, and W. Ho, Phys. Rev. Lett. 82, 1724-1727 (1999).



Site Specific Displacement of Si Adatoms on Si(111)-(7x7), B.C. Stipe, M.A. Rezaei, and W. Ho, Phys. Rev. Lett. 79, 4397-4400 (1997).


Inducing and Imaging Single Molecule Dissociation on a Semiconductor Surface: H2S and D2S on Si(111)-7x7, M.A. Rezaei, B.C. Stipe, and W. Ho, J. Chem. Phys. 109, 6075-6078 (1998). Atomically Resolved Determination of the Adsorption Sites as a Function of Temperature and Coverage: H2S on Si(111)-7x7, M.A. Rezaei, B.C. Stipe, and W. Ho, J. Phys. Chem. 102, 10941-10947 (1998). Imaging the Atomically Resolved Dissociation of D2S on Si(100) from 80 to 300 K, M.A. Rezaei, B.C. Stipe, and W. Ho, J. Chem. Phys. 110, 3548-3552 (1999).


Atomically Resolved Adsorption and Scanning Tunneling Microscope Induced Desorption on a Semiconductor: NO on Si(111)-7x7, M.A. Rezaei, B.C. Stipe, and W. Ho, J. Chem. Phys. 110, 4891-4896 (1999).


Vibrational Analysis of Single Molecule Chemistry: Ethylene Dehydrogenation on Ni(110), J. Gaudioso, H.J. Lee, and W. Ho, J. Am. Chem. Soc. 121, 8479-8485 (1999).


Single-molecule Vibrational Spectroscopy and Microscopy: CO on Cu(001) adn Cu(110), L.J. Lauhon and W. Ho, Phys. Rev. B 60, R8525-R8528 (1999).


Single-molecule Thermal Rotation and Diffusion: Acetylene on Cu(001), L.J. Lauhon and W. Ho, J. Chem. Phys. 111, 5633-5636 (1999).


Single Bond Formation and Characterization with a Scanning Tunneling Microscope, H.J. Lee and W. Ho, Science 286, 1719-1722 (1999).


Control and Characterization of a Multistep Unimolecular Reaction, L.J. Lauhon and W. Ho, Phys. Rev. Lett. 84, 1527-1530 (2000).


Single Molecule Chemistry and Vibrational Spectroscopy: Pyridine and Benzene on Cu(001), L.J. Lauhon and W. Ho, J. Phys. Chem. A 104, 2463-2467 (2000).


Electronic and Vibrational Excitation of Single Molecules with a Scanning Tunneling Microscope, L.J. Lauhon and W. Ho, Surf. Sci. 451, 219-225 (2000).


Structural Determination by Single-Molecule Vibrational Spectroscopy and Microscopy: Contrast Between Copper and Iron Carbonyls, H.J. Lee and W. Ho, Phys. Rev. B 61, R16347-R16350 (2000).


Electronic Resonance and Symmetry in Single-Molecule Inelastic Electron Tunneling, J.R. Hahn, H.J. Lee, and W. Ho, Phys. Rev. Lett. (2000).


Vibrationally Mediated Negative Differential Resistance in a Single Molecule, J. Gaudioso, L.J. Lauhon, and W. Ho, Phys. Rev. Lett. (2000).


Single Molecule Vibrational Spectroscopy and Microscopy: Cu(II) Etioporphyrin-I on Cu(001), T.M. Wallis, X. Chen, and W. Ho, J. Chem. Phys. Commun. (2000).


Last modified: August 8, 2000

Douglas E. Milton, Sr., dem8@cornell.edu