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Publications

Coexisting ferromagnetic–antiferromagnetic state in twisted bilayer CrI3

Cornell Affiliated Author(s)
Author
Y. Xu
A. Ray
Y.-T. Shao
S. Jiang
K. Lee
D. Weber
J.E. Goldberger
K. Watanabe
T. Taniguchi
D.A. Muller
K.F. Mak
J. Shan
Abstract

Moiré engineering1–3 of van der Waals magnetic materials4–9 can yield new magnetic ground states via competing interactions in moiré superlattices10–13. Theory predicts a suite of interesting phenomena, including multiflavour magnetic states10, non-collinear magnetic states10–13, moiré magnon bands and magnon networks14 in twisted bilayer magnetic crystals, but so far such non-trivial magnetic ground states have not emerged experimentally.

Journal
Nature Nanotechnology
Date Published
Funding Source
DMR-1807810
FA9550-18-1-0480
FA9550-19-1-0390
DMR-1719875
DMR-2011876
WE6480/1
JPMJCR15F3
Group (Lab)
Jie Shan Group
Kin Fai Mak Group

Valley-Polarized Quantum Anomalous Hall State in Moiré MoTe2/WSe2 Heterobilayers

Cornell Affiliated Author(s)
Author
Y.-M. Xie
C.-P. Zhang
J.-X. Hu
K.F. Mak
K.T. Law
Abstract

Moiré heterobilayer transition metal dichalcogenides (TMDs) emerge as an ideal system for simulating the single-band Hubbard model and interesting correlated phases have been observed in these systems. Nevertheless, the moiré bands in heterobilayer TMDs were believed to be topologically trivial. Recently, it was reported that both a quantum valley Hall insulating state at filling ν=2 (two holes per moiré unit cell) and a valley-polarized quantum anomalous Hall state at filling ν=1 were observed in AB stacked moiré MoTe2/WSe2 heterobilayers.

Journal
Physical Review Letters
Date Published
Funding Source
FA9550-20-1-0219
16309718
16310219
16310520
AoE/P-701/20
C6025-19G
RFS2021-6S03
Group (Lab)
Kin Fai Mak Group

Quantum anomalous Hall effect from intertwined moiré bands

Cornell Affiliated Author(s)
Author
T. Li
S. Jiang
B. Shen
Y. Zhang
L. Li
Z. Tao
T. Devakul
K. Watanabe
T. Taniguchi
L. Fu
J. Shan
K.F. Mak
Abstract

Electron correlation and topology are two central threads of modern condensed matter physics. Semiconductor moiré materials provide a highly tuneable platform for studies of electron correlation1–12. Correlation-driven phenomena, including the Mott insulator2–5, generalized Wigner crystals2,6,9, stripe phases10 and continuous Mott transition11,12, have been demonstrated. However, non-trivial band topology has remained unclear. Here we report the observation of a quantum anomalous Hall effect in AB-stacked MoTe2 /WSe2 moiré heterobilayers.

Journal
Nature
Date Published
Funding Source
NNCI-1542081
FA9550-19-1-0390
FA9550-20-1-0219
W911NF-17-1-0605
DE-SC0019481
DE-SC0020149
DMR-1719875
JPMJCR15F3
Group (Lab)
Jie Shan Group
Kin Fai Mak Group

Quantum Oscillations in Two-Dimensional Insulators Induced by Graphite Gates

Cornell Affiliated Author(s)
Author
J. Zhu
T. Li
A.F. Young
J. Shan
K.F. Mak
Abstract

We demonstrate a mechanism for magnetoresistance oscillations in insulating states of two-dimensional (2D) materials arising from the interaction of the 2D layer and proximal graphite gates. We study a series of devices based on different 2D systems, including mono- and bilayer Td-WTe2, MoTe2/WSe2 moiré heterobilayers, and Bernal-stacked bilayer graphene, which all share a similar graphite-gated geometry.

Journal
Physical Review Letters
Date Published
Funding Source
DMR-2039380
N00014-20-1-2609
W911NF-17-1-0605
GBMF9471
DMR-1719875
Group (Lab)
Jie Shan Group
Kin Fai Mak Group

Strongly correlated excitonic insulator in atomic double layers

Cornell Affiliated Author(s)
Author
L. Ma
P.X. Nguyen
Z. Wang
Y. Zeng
K. Watanabe
T. Taniguchi
A.H. MacDonald
K.F. Mak
J. Shan
Abstract

Excitonic insulators (EIs) arise from the formation of bound electron–hole pairs (excitons)1,2 in semiconductors and provide a solid-state platform for quantum many-boson physics3–8. Strong exciton–exciton repulsion is expected to stabilize condensed superfluid and crystalline phases by suppressing both density and phase fluctuations8–11. Although spectroscopic signatures of EIs have been reported6,12–14, conclusive evidence for strongly correlated EI states has remained elusive.

Journal
Nature
Date Published
Funding Source
DMR-2004451
N00014-21-1-2471
DE-SC0019481
DE-SC0022058
NNCI-2025233
JPMJCR15F3
Group (Lab)
Jie Shan Group
Kin Fai Mak Group

Air-Stable and Layer-Dependent Ferromagnetism in Atomically Thin van der Waals CrPS4

Cornell Affiliated Author(s)
Author
J. Son
S. Son
P. Park
M. Kim
Z. Tao
J. Oh
T. Lee
S. Lee
J. Kim
K. Zhang
K. Cho
T. Kamiyama
J.H. Lee
K.F. Mak
J. Shan
M. Kim
J.-G. Park
J. Lee
Abstract

Ferromagnetism in two-dimensional materials presents a promising platform for the development of ultrathin spintronic devices with advanced functionalities. Recently discovered ferromagnetic van der Waals crystals such as CrI3, readily isolated two-dimensional crystals, are highly tunable through external fields or structural modifications. However, there remains a challenge because of material instability under air exposure. Here, we report the observation of an air-stable and layer-dependent ferromagnetic (FM) van der Waals crystal, CrPS4, using magneto-optic Kerr effect microscopy.

Journal
ACS Nano
Date Published
Funding Source
DMR-1807810
2017R1C1B2002631
2020R1A2C2011334
2020R1A5A6052558
2021R1A5A1032996
2017M3D1A1040828
2017R1A2B3011629
2020R1A3B2079375
IBS-R009-G1
Group (Lab)
Jie Shan Group
Kin Fai Mak Group

Charge-order-enhanced capacitance in semiconductor moiré superlattices

Cornell Affiliated Author(s)
Author
T. Li
J. Zhu
Y. Tang
K. Watanabe
T. Taniguchi
V. Elser
J. Shan
K.F. Mak
Abstract

Van der Waals moiré materials have emerged as a highly controllable platform to study electronic correlation phenomena1–17. Robust correlated insulating states have recently been discovered at both integer and fractional filling factors of semiconductor moiré systems10–17. In this study we explored the thermodynamic properties of these states by measuring the gate capacitance of MoSe2/WS2 moiré superlattices. We observed a series of incompressible states for filling factors 0–8 and anomalously large capacitance in the intervening compressible regions.

Journal
Nature Nanotechnology
Date Published
Funding Source
FA9550-18-1-0480
DMR-1539918
NNCI-1542081
DE-SC0019481
JPMJCR15F3
Group (Lab)
Jie Shan Group
Kin Fai Mak Group
Veit Elser Group

Continuous Mott transition in semiconductor moiré superlattices

Author
T. Li
S. Jiang
L. Li
Y. Zhang
K. Kang
J. Zhu
K. Watanabe
T. Taniguchi
Debanjan Chowdhury
L. Fu
J. Shan
K.F. Mak
Abstract

The evolution of a Landau Fermi liquid into a non-magnetic Mott insulator with increasing electronic interactions is one of the most puzzling quantum phase transitions in physics1–6. The vicinity of the transition is believed to host exotic states of matter such as quantum spin liquids4–7, exciton condensates8 and unconventional superconductivity1. Semiconductor moiré materials realize a highly controllable Hubbard model simulator on a triangular lattice9–22, providing a unique opportunity to drive a metal–insulator transition (MIT) via continuous tuning of the electronic interactions.

Journal
Nature
Date Published
Funding Source
DMR-1807810
W911NF-17-1-0605
DMR-1719875
NNCI-1542081
JPMJCR15F3
Group (Lab)
Debanjan Chowdhury Group
Jie Shan Group
Kin Fai Mak Group

Two-fold symmetric superconductivity in few-layer NbSe2

Cornell Affiliated Author(s)
Author
A. Hamill
B. Heischmidt
E. Sohn
D. Shaffer
K.-T. Tsai
X. Zhang
X. Xi
A. Suslov
H. Berger
L. Forró
F.J. Burnell
J. Shan
K.F. Mak
R.M. Fernandes
K. Wang
V.S. Pribiag
Abstract

The strong Ising spin–orbit coupling in certain two-dimensional transition metal dichalcogenides can profoundly affect the superconducting state in few-layer samples. For example, in NbSe2, this effect combines with the reduced dimensionality to stabilize the superconducting state against magnetic fields up to 35 T, and could lead to topological superconductivity. Here we report a two-fold rotational symmetry of the superconducting state in few-layer NbSe2 under in-plane external magnetic fields, in contrast to the three-fold symmetry of the lattice.

Journal
Nature Physics
Date Published
Funding Source
DMR-2011401
2011401
DMR-1420013
DMR-1644779
DMR-1807810
ECCS-1542202
N00014-18-1-2368
Group (Lab)
Jie Shan Group
Kin Fai Mak Group

Stripe phases in WSe2/WS2 moiré superlattices

Cornell Affiliated Author(s)
Author
C. Jin
Z. Tao
T. Li
Y. Xu
Y. Tang
J. Zhu
S. Liu
K. Watanabe
T. Taniguchi
J.C. Hone
L. Fu
J. Shan
K.F. Mak
Abstract

Stripe phases, in which the rotational symmetry of charge density is spontaneously broken, occur in many strongly correlated systems with competing interactions1–11. However, identifying and studying such stripe phases remains challenging. Here we uncover stripe phases in WSe2/WS2 moiré superlattices by combining optical anisotropy and electronic compressibility measurements. We find strong electronic anisotropy over a large doping range peaked at 1/2 filling of the moiré superlattice. The 1/2 state is incompressible and assigned to an insulating stripe crystal phase.

Journal
Nature Materials
Date Published
Funding Source
N00014-18-1-2368 Here
FA9550-20-1-0219
DE-SC0019481
W911NF-17-1-0605
JPMJCR15F3
Group (Lab)
Jie Shan Group
Kin Fai Mak Group