Skip to main content

Publications

Avoided valence transition in a plutonium superconductor

Cornell Affiliated Author(s)
Author
B. Ramshaw
Arkady Shekhter
Ross McDonald
Jon Betts
J. Mitchell
P. Tobash
C. Mielke
E. Bauer
Albert Migliori
Abstract

The d and f electrons in correlated metals are often neither fully localized around their host nuclei nor fully itinerant. This localized/itinerant duality underlies the correlated electronic states of the high-Tc cuprate superconductors and the heavy-fermion intermetallics and is nowhere more apparent than in the 5f valence electrons of plutonium. Here, we report the full set of symmetry-resolved elastic moduli of PuCoGa5 - the highest Tc superconductor of the heavy fermions (Tc = 18.5 K) - and find that the bulk modulus softens anomalously over a wide range in temperature above Tc.

Journal
Proceedings of the National Academy of Sciences of the United States of America
Date Published
Funding Source
DMR-1157490
Group (Lab)
Brad Ramshaw Group

Evidence for a small hole pocket in the Fermi surface of underdoped YBa2Cu3Oy

Cornell Affiliated Author(s)
Author
N. Doiron-Leyraud
S. Badoux
S. René de Cotret
S. Lepault
D. LeBoeuf
Francis Laliberté
Elena Hassinger
B. Ramshaw
D. Bonn
W. Hardy
R. Liang
J.-H.. Park
D. Vignolles
B. Vignolle
L. Taillefer
C. Proust
Abstract

In underdoped cuprate superconductors, the Fermi surface undergoes a reconstruction that produces a small electron pocket, but whether there is another, as yet, undetected portion to the Fermi surface is unknown. Establishing the complete topology of the Fermi surface is key to identifying the mechanism responsible for its reconstruction. Here we report evidence for a second Fermi pocket in underdoped YBa2Cu3Oy, detected as a small quantum oscillation frequency in the thermoelectric response and in the c-axis resistance.

Journal
Nature Communications
Date Published
Group (Lab)
Brad Ramshaw Group

Direct measurement of the upper critical field in cuprate superconductors

Cornell Affiliated Author(s)
Author
Gael Grissonnanche
Olivier Cyr-Choinière
Francis Laliberté
S. René de Cotret
A. Juneau-Fecteau
S. Dufour-Beauséjour
M.-È. Delage
D. LeBoeuf
J. Chang
B.J. Ramshaw
D.A. Bonn
W.N. Hardy
R. Liang
S. Adachi
N.E. Hussey
B. Vignolle
C. Proust
M. Sutherland
S. Krämer
J.-H. Park
D. Graf
N. Doiron-Leyraud
L. Taillefer
Abstract

In the quest to increase the critical temperature Tc of cuprate superconductors, it is essential to identify the factors that limit the strength of superconductivity. The upper critical field Hc2 is a fundamental measure of that strength, yet there is no agreement on its magnitude and doping dependence in cuprate superconductors. Here we show that the thermal conductivity can be used to directly detect Hc2 in the cuprates YBa2Cu3Oy, YBa2Cu4O8 and Tl2Ba2CuO6+δ, allowing us to map out Hc2 across the doping phase diagram.

Journal
Nature Communications
Date Published
Group (Lab)
Brad Ramshaw Group

Bounding the pseudogap with a line of phase transitions in YBa2 Cu3 O 6+δ

Cornell Affiliated Author(s)
Author
A. Shekhter
B.J. Ramshaw
R. Liang
W.N. Hardy
D.A. Bonn
Fedor Balakirev
R.D. McDonald
Jon Betts
S.C. Riggs
A. Migliori
Abstract

Close to optimal doping, the copper oxide superconductors show 'strange metal' behaviour, suggestive of strong fluctuations associated with a quantum critical point. Such a critical point requires a line of classical phase transitions terminating at zero temperature near optimal doping inside the superconducting 'dome'.

Journal
Nature
Date Published
Group (Lab)
Brad Ramshaw Group

Vortex lattice melting and H c2 in underdoped YBa 2Cu 3O y

Cornell Affiliated Author(s)
Author
B. Ramshaw
James Day
Baptiste Vignolle
David LeBoeuf
P. Dosanjh
Cyril Proust
Louis Taillefer
Ruixing Liang
W. Hardy
D. Bonn
Abstract

Vortices in a type-II superconductor form a lattice structure that melts when the thermal displacement of the vortices is an appreciable fraction of the distance between vortices. In an anisotropic high-T c superconductor, such as YBa 2Cu 3O y, the magnetic field value where this melting occurs can be much lower than the mean-field critical field H c2. We examine this melting transition in YBa 2Cu 3O y with oxygen content y from 6.45 to 6.92, and we perform a quantitative analysis of this transition in the cuprates by fitting the data to a theory of vortex-lattice melting.

Journal
Physical Review B - Condensed Matter and Materials Physics
Date Published
Group (Lab)
Brad Ramshaw Group

Coherent c-axis transport in the underdoped cuprate superconductor YBa 2Cu 3O y

Cornell Affiliated Author(s)
Author
B. Vignolle
B.J. Ramshaw
J. Day
D. LeBoeuf
S. Lepault
R. Liang
W.N. Hardy
D.A. Bonn
L. Taillefer
C. Proust
Abstract

The electrical resistivity Ï c of the underdoped cuprate superconductor YBa 2Cu 3O y was measured perpendicular to the CuO 2 planes on ultrahigh quality single crystals in magnetic fields large enough to suppress superconductivity. The incoherent insulating-like behavior of Ï c at high temperature, characteristic of all underdoped cuprates, is found to cross over to a coherent regime of metallic behavior at low temperature.

Journal
Physical Review B - Condensed Matter and Materials Physics
Date Published
Group (Lab)
Brad Ramshaw Group

Fermi-surface reconstruction by stripe order in cuprate superconductors

Cornell Affiliated Author(s)
Author
Francis Laliberté
J. Chang
N. Doiron-Leyraud
Elena Hassinger
R. Daou
M. Rondeau
B.J. Ramshaw
R. Liang
D.A. Bonn
W.N. Hardy
S. Pyon
T. Takayama
H. Takagi
I. Sheikin
L. Malone
C. Proust
K. Behnia
Louis Taillefer
Abstract

The origin of pairing in a superconductor resides in the underlying normal state. In the cuprate high-temperature superconductor YBa2Cu 3Oy (YBCO), application of a magnetic field to suppress superconductivity reveals a ground state that appears to break the translational symmetry of the lattice, pointing to some density-wave order. Here we use a comparative study of thermoelectric transport in the cuprates YBCO and La 1.8-xEu0.2SrxCuO4(Eu-LSCO) to show that the two materials exhibit the same process of Fermi-surface reconstruction as a function of temperature and doping.

Journal
Nature Communications
Date Published
Group (Lab)
Brad Ramshaw Group

Nernst effect in the cuprate superconductor YBa2Cu 3Oy: Broken rotational and translational symmetries

Cornell Affiliated Author(s)
Author
J. Chang
Nicolas Doiron-Leyraud
Francis Laliberté
R. Daou
David LeBoeuf
B. Ramshaw
Ruixing Liang
D. Bonn
W. Hardy
Cyril Proust
I. Sheikin
K. Behnia
Louis Taillefer
Abstract

The Nernst coefficient of the cuprate superconductor YBa2Cu 3Oy was recently shown to become strongly anisotropic within the basal plane when cooled below the pseudogap temperature T, revealing that the pseudogap phase breaks the fourfold rotational symmetry of the CuO 2 planes. Here we report on the evolution of this Nernst anisotropy at low temperature, once superconductivity is suppressed by a magnetic field. We find that the anisotropy drops rapidly below 80 K, to vanish in the T=0 limit.

Journal
Physical Review B - Condensed Matter and Materials Physics
Date Published
Group (Lab)
Brad Ramshaw Group