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Publications

Elastocaloric determination of the phase diagram of Sr2RuO4

Cornell Affiliated Author(s)
Author
Y.-S. Li
M. Garst
J. Schmalian
S. Ghosh
N. Kikugawa
D.A. Sokolov
C.W. Hicks
F. Jerzembeck
M.S. Ikeda
Z. Hu
B.J. Ramshaw
A.W. Rost
M. Nicklas
A.P. Mackenzie
Abstract

One of the main developments in unconventional superconductivity in the past two decades has been the discovery that most unconventional superconductors form phase diagrams that also contain other strongly correlated states. Many systems of interest are therefore close to more than one instability, and tuning between the resultant ordered phases is the subject of intense research1.

Journal
Nature
Date Published
Group (Lab)
Brad Ramshaw Group

Strong magnetoelastic coupling in Mn3X (X=Ge, Sn)

Cornell Affiliated Author(s)
Author
Florian Theuss
Sayak Ghosh
Taishi Chen
Oleg Tchernyshyov
Satoru Nakatsuji
B. Ramshaw
Abstract

We measure the full elastic tensors of Mn3Ge and Mn3Sn as a function of temperature through their respective antiferromagnetic phase transitions. Large discontinuities in the bulk moduli at the Néel transitions indicate strong magnetoelastic coupling in both compounds. Strikingly, the discontinuities are nearly a factor of 10 larger in Mn3Ge than in Mn3Sn. We use the magnitudes of the discontinuities to calculate the pressure derivatives of the Néel temperature, which are 39 K/GPa 14.3 K/GPa for Mn3Ge and Mn3Sn, respectively.

Journal
Physical Review B
Date Published
Group (Lab)
Brad Ramshaw Group

Fermi surface transformation at the pseudogap critical point of a cuprate superconductor

Author
Yawen Fang
Gael Grissonnanche
Anaëlle Legros
Simon Verret
Francis Laliberté
C. Collignon
Amirreza Ataei
Maxime Dion
Jianshi Zhou
David Graf
Michael Lawler
Paul Goddard
Louis Taillefer
B. Ramshaw
Abstract

The nature of the pseudogap phase remains a major puzzle in our understanding of cuprate high-temperature superconductivity. Whether or not this metallic phase is defined by any of the reported broken symmetries, the topology of its Fermi surface remains a fundamental open question. Here we use angle-dependent magnetoresistance (ADMR) to measure the Fermi surface of the La1.6–xNd0.4SrxCuO4 cuprate. Outside the pseudogap phase, we fit the ADMR data and extract a Fermi surface geometry that is in excellent agreement with angle-resolved photoemission data.

Journal
Nature Physics
Date Published
Group (Lab)
Brad Ramshaw Group
Michael Lawler Group

Weyl Fermion magneto-electrodynamics and ultralow field quantum limit in TaAs

Cornell Affiliated Author(s)
Author
Zhengguang Lu
Patrick Hollister
Mykhaylo Ozerov
Seongphill Moon
Eric Bauer
Filip Ronning
Dmitry Smirnov
Long Ju
B. Ramshaw
Abstract

Topological semimetals are predicted to exhibit unconventional electrodynamics, but a central experimental challenge is singling out the contributions from the topological bands. TaAs is the prototypical example, where 24 Weyl points and 8 trivial Fermi surfaces make the interpretation of any experiment in terms of band topology ambiguous. We report magneto-infrared reflection spectroscopy measurements on TaAs. We observed sharp inter-Landau level transitions from a single pocket of Weyl Fermions in magnetic fields as low as 0.4 tesla.

Journal
Science Advances
Date Published
Group (Lab)
Brad Ramshaw Group

Quantum oscillations and quasiparticle properties of thin film

Cornell Affiliated Author(s)
Author
Yawen Fang
Hari Nair
Ludi Miao
Berit Goodge
Nathaniel Schreiber
Jacob Ruf
Lena Kourkoutis
Kyle Shen
Darrell Schlom
B. Ramshaw
Abstract

We measure the Shubnikov-de Haas effect in thin-film grown on an substrate. We detect all three known Fermi surfaces and extract the Fermi surface volumes, cyclotron effective masses, and quantum lifetimes. We show that the electronic structure is nearly identical to that of single-crystal , and that the quasiparticle lifetime is consistent with the of comparably clean, single-crystal . Unlike single-crystal , where the quantum and transport lifetimes are roughly equal, we find that the transport lifetime is times longer than the quantum lifetime.

Journal
Physical Review B
Date Published
Funding Source
DMR-1709255
DGE-1650441
DMR-1539918
1429155
DMR-1644779
DMR-1752784
NNCI-2025233
FA9550-15-1-0474
GBMF3850
GBMF9073
DMR-1719875
Group (Lab)
Brad Ramshaw Group
Kyle Shen Group

Linear-in temperature resistivity from an isotropic Planckian scattering rate

Cornell Affiliated Author(s)
Author
Gael Grissonnanche
Yawen Fang
Anaëlle Legros
Simon Verret
Francis Laliberté
C. Collignon
Jianshi Zhou
David Graf
Paul Goddard
Louis Taillefer
B. Ramshaw
Abstract

A variety of ‘strange metals’ exhibit resistivity that decreases linearly with temperature as the temperature decreases to zero1–3, in contrast to conventional metals where resistivity decreases quadratically with temperature. This linear-in-temperature resistivity has been attributed to charge carriers scattering at a rate given by ħ/τ = αkBT, where α is a constant of order unity, ħ is the Planck constant and kB is the Boltzmann constant.

Journal
Nature
Date Published
Group (Lab)
Brad Ramshaw Group

Remarkably Weak Anisotropy in Thermal Conductivity of Two-Dimensional Hybrid Perovskite Butylammonium Lead Iodide Crystals

Cornell Affiliated Author(s)
Author
Chen Li
Hao Ma
Tianyang Li
Jinghang Dai
Md. Rasel
Alessandro Mattoni
Ahmet Alatas
Malcolm Thomas
Zachary Rouse
Avi Shragai
Shefford Baker
B. Ramshaw
Joseph Feser
David Mitzi
Zhiting Tian
Abstract

Two-dimensional (2D) hybrid organic-inorganic perovskites consisting of alternating organic and inorganic layers are a new class of layered structures. They have attracted increasing interest for photovoltaic, optoelectronic, and thermoelectric applications, where knowing their thermal transport properties is critical. We carry out both experimental and computational studies on thermal transport properties of 2D butylammonium lead iodide crystals and find their thermal conductivity is ultralow (below 0.3 W m-1 K-1) with very weak anisotropy (around 1.5) among layered crystals.

Journal
Nano Letters
Date Published
Funding Source
ACI-1053575
CBET1839384
NNCI-2025233
DE-AC36-08G028308
DE-AC02-06CH11357
DMR-1719875
Group (Lab)
Brad Ramshaw Group

Scale-invariant magnetic anisotropy in RuCl3 at high magnetic fields

Cornell Affiliated Author(s)
Author
K. Modic
Ross McDonald
J. Ruff
Maja Bachmann
You Lai
Johanna Palmstrom
David Graf
Mun Chan
Fedor Balakirev
Jon Betts
G.S. Boebinger
Marcus Schmidt
Michael Lawler
D. Sokolov
Philip Moll
B. Ramshaw
Arkady Shekhter
Abstract

In RuCl3, inelastic neutron scattering and Raman spectroscopy reveal a continuum of non-spin-wave excitations that persists to high temperature, suggesting the presence of a spin liquid state on a honeycomb lattice. In the context of the Kitaev model, finite magnetic fields introduce interactions between the elementary excitations, and thus the effects of high magnetic fields that are comparable to the spin-exchange energy scale must be explored.

Journal
Nature Physics
Date Published
Funding Source
DMR-1157490
DMR-1644779
1157490
1332208
Group (Lab)
Brad Ramshaw Group
Michael Lawler Group

Thermodynamic evidence for a two-component superconducting order parameter in Sr2RuO4

Cornell Affiliated Author(s)
Author
Sayak Ghosh
Arkady Shekhter
F. Jerzembeck
N. Kikugawa
Dmitry Sokolov
Manuel Brando
A. Mackenzie
Clifford Hicks
B. Ramshaw
Abstract

Sr2RuO4 has stood as the leading candidate for a spin-triplet superconductor for 26 years1. However, recent NMR experiments have cast doubt on this candidacy2,3 and it is difficult to find a theory of superconductivity that is consistent with all experiments. The order parameter symmetry for this material therefore remains an open question. Symmetry-based experiments are needed that can rule out broad classes of possible superconducting order parameters.

Journal
Nature Physics
Date Published
Group (Lab)
Brad Ramshaw Group

Superconductivity and quantum criticality linked by the Hall effect in a strange metal

Cornell Affiliated Author(s)
Author
Ian Hayes
Nikola Maksimovic
Gilbert Lopez
Mun Chan
B. Ramshaw
Ross McDonald
James Analytis
Abstract

Many unconventional superconductors exhibit a common set of anomalous charge transport properties that characterize them as ‘strange metals’, which provides hope that there is a single theory that describes them1–3. However, model-independent connections between the strange metals and superconductivity have remained elusive. Here, we show that the Hall effect of the unconventional superconductor BaFe2(As1−xPx)2 contains an anomalous contribution arising from the correlations within the strange metal.

Journal
Nature Physics
Date Published
Funding Source
DMR-1157490
DMR-1644779
GBMF9067
DE-AC02-05CH11231
Group (Lab)
Brad Ramshaw Group