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Probing many-body interactions in monolayer transition-metal dichalcogenides

Cornell Affiliated Author(s)

Author

D. Van Tuan
B. Scharf
Z. Wang
J. Shan
K.F. Mak
I. Žutić
H. Dery

Abstract

Many-body interactions in monolayer transition-metal dichalcogenides are strongly affected by their unique band structure. We study these interactions by measuring the energy shift of neutral excitons (bound electron-hole pairs) in gated WSe2 and MoSe2. Surprisingly, while the blueshift of the neutral exciton X0 in electron-doped samples can be more than 10 meV, the blueshift in hole-doped samples is nearly absent. Taking into account dynamical screening and local-field effects, we present a transparent and analytical model that elucidates the crucial role played by intervalley plasmons in electron-doped conditions. The energy shift of X0 as a function of charge density is computed showing agreement with experiment, where the renormalization of X0 by intervalley plasmons yields a stronger blueshift in MoSe2 than in WSe2 due to differences in their band ordering. © 2019 American Physical Society.

Date Published

Journal

Physical Review B

Volume

99

Issue

8

URL

https://www.scopus.com/inward/record.uri?eid=2-s2.0-85061446043&doi=10.1103%2fPhysRevB.99.085301&partnerID=40&md5=e034007d0fcbf96a8884dec7e8a24c5c

DOI

10.1103/PhysRevB.99.085301

Group (Lab)

Jie Shan Group
Kin Fai Mak Group

Funding Source

N000141712793
1410407
1503601
DESC0012635
DESC0013883

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